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Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications

Yıl 2019, Cilt: 13 Sayı: 37, 1 - 8, 26.05.2019

Busra Tandogan Gizem Eker Sanlı

Öz

The aim of this study was to investigate the removal of polychlorinated biphenyl (PCB) compounds from the soil samples taken from around a cement plant in Bursa-Turkey. Ambient air applications were carried out, and the effects of titanium dioxide (TiO2), diethylamine (DEA) and hydrogen peroxide (H2O2) on the removal of PCBs were determined. Firstly, the soil samples without any additives were exposed to ambient air conditions for 24 hours. Then, TiO2, DEA and H2O2 were added to the soils at 1%, 10% and 20% of the soil dry weight. The PCB concentrations were measured using a gas chromatography-electron capture detector (GC-ECD). Only 2% Σ82 PCB removal efficiency was obtained in the sample prepared without using additive. This value reached 86% when 10% DEA was used as an additive. It was concluded that sunlight was not effective in the degradation of PCBs in soil without the use of additives and DEA was the most efficient photocatalyst for this study. Among the all ambient air applications, the 4- and 5- chlorine homolog group compounds were removed at the maximum ratio, while the 8- and 9- chlorine homolog group showed the lowest removal efficiency.

Anahtar Kelimeler

TiO2 DEA H2O2 Soil Sunlight Photodegradation

Kaynakça

  • Ahmad M, Simon MA, Sherrin A, Tuccillo ME, Ullman JL, Teel AL and Watts RJ (2011). Treatment of polychlorinated biphenyls in two surface soils using catalyzed H2O2 propagations. Chemosphere 84:855-862.
  • Brawn J F BDL, Brennan M J, Carnahan J C, Feng H, Wanger R E (1987). Polychlorinated Biphenyl Dechlorination in Aquatic Sediment. Science 236:709-712.
  • Bunce NJ, Kumar Y, Ravanal L, Safe S (1978). Cosmochemistry of chlorinated biphenyl's in ISO-octane solution. Journal of the Chemical Society-Perkins Transactions 2:880-884.
  • Cebe M (1995). Physicochemistry Volume II: Fundamental Concepts in Reaction Kinetics. Uludag University Press, Turkey.
  • Cetin B (2016). Investigation of Paths, PCBs and PCNs in soils around a Heavily Industrialized Area in Kocaeli, Turkey: Concentrations, distributions, sources and toxicological effects. Science of the Total Environment 560:160-169.
  • Dhol A (2005). An Investigation of a Photochemical Approach for the Remediation of PCB-Contaminated Soils. Master Thesis. University of Calgary, Canada.
  • Dong D, Li P, Xiaojun I, Xu C (2010). Photocatalytic degradation of phenanthrene and pyrene on soil surfaces in the presence of nanometer rutile TiO2 under UV-irradiation. Chemical Engineering Journal 158:378-383.
  • Dönmez B (2012). Research of Polychlorinated Biphenyl (PCB) Pollution in Soil Samples and Evaluation of Applicability of Limit Values. Master Thesis. Istanbul Technical University, Turkey.
  • Fasnacht MP and Blough NV (2003). Mechanisms of the aqueous photodegradation of polycyclic aromatic hydrocarbons. Environ Sci Technol 37:5767-5772.
  • Garcia R, Diaz-Somoano M, Calvo M, Lopez-Anton MA, Suarez S, Ruiz IS, Martinez-Tarazona MR (2012). Impact of a semi-industrial coke processing plant in the surrounding surface soil. Part II: PAH content Fuel Process Technol 104:245-252.
  • Guieysse B, Viklund G, Toes AC, Mattiasson B (2004). Combined UV-biological degradation of PAHs. Chemosphere 55:1493-1499.
  • Hoffmann MR, Martin ST, Choi WY, Bahnemann DW (1995). Environmental Applications of Semiconductor Photocatalysis. Chem Rev 95:69-96.
  • Ireland JC, Davila B, Moreno H, Fink SK, Tassos S (1995). Heterogeneous Photocatalytic Decomposition of Polyaromatic Hydrocarbons over Titanium-Dioxide. Chemosphere 30:965-984.
  • Jelic A, Di Fabio S, Vecchiato G, Cecchi F, Fatone F (2015). Nano-occurrence and removal of PCBs within the Europe's largest petrochemical MBR system. Water Research 83:329-336.
  • Karaca G (2013). Determination of Polycyclic Aromatic Hydrocarbon (PAHs) Levels in Treatment Sludge, Nilüfer Creek Sediment and Investigation of Removal Methods. Uludag University, Turkey.
  • Karaca G, Cindoruk SS, Tasdemir Y (2014). Migration of polycyclic aromatic hydrocarbons (PAHs) in urban treatment sludge to the air during PAH removal applications. J Air Waste Manage 64:568-577.
  • Karaca G and Tasdemir Y (2011). Effect of Diethylamine on Pah Removal from Municipal Sludge under UV Light. Fresenius Environmental Bulletin 20:1777-1784.
  • Karaca G and Tasdemir Y (2015). Application of Advanced Oxidation Processes for Polycyclic Aromatic Hydrocarbons Removal from Municipal Treatment Sludge. Clean-Soil Air Water 43:191-196.
  • Karaca G and Taşdemir Y (2015). Removal of Polycyclic Aromatic Hydrocarbons (PAHs) From Organizated Industry Dıstrıct Treatment Sludges With Photochemical Degradation: Ambient Air Applications. Journal of the Faculty of Engineering and Architecture of Gazi University 30:557-565.
  • Krauss M and Wilcke W (2002). Photochemical oxidation of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in soils - a tool to assess their degradability. J Plant Nutr Soil Sc 165:173-178.
  • Lin X, Jin Y, Wu H, Chen T, Li X, Lu S, Jiang X and Yan J (2013). Removal of PCDD/Fs and PCBs from flue gas using a pilot gas cleaning system. Journal of Environmental Sciences 25:1833-1840.
  • Lin YJ, Gupta G, Baker J (1995). Photodegradation of Polychlorinated Biphenyl Congeners Using Simulated Sunlight and Diethylamine. Chemosphere 31:3323-3344.
  • Lin YJ, Teng LS, Lee A, Chen YL (2004). Effect of photosensitizer diethylamine on the photodegradation of polychlorinated biphenyls. Chemosphere 55:879-884.
  • Meijer SN, Ockenden WA, Sweetman A, Breivik K, Grimalt JO, Jones KC (2003). Global distribution and budget of PCBs and CB in background surface soils: Implications for sources and environmental processes. Environ Sci Technol 37:667-672.
  • Melnyk A, Dettlaff A, Kuklinska K, Namiesnik J, Wolska L (2015). Concentration and sources of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in surface soil near a municipal solid waste (MSW) landfill. Science of the Total Environment 530:18-27.
  • Miller JS and Olejnik D (2001). Photolysis of polycyclic aromatic hydrocarbons in water. Water Res 35:233-243.
  • Ogulmus R (2012). Territories Polychlorinated Biphenyls (PCBs) Regional and Seasonal Conditions. Master Thesis. Uludag University, Turkey.
  • Ortiz R, Vega S, Gutierrez R, Gibson R, Schettino B and Ramirez ML (2012). Presence of Polycyclic Aromatic Hydrocarbons (PAHs) in Top Soils from Rural Terrains in Mexico City. Bulletin of Environmental Contamination and Toxicology 88:428-432.
  • Pleskov YV, Fujishima A, Hashimoto K and Watanabe T (1999). TiO2 photocatalysis: Fundamentals and applications, Tokyo: Bks, Inc., Russ. J Electrochem 35:1137-1138.
  • Quan X, Zhao X, Chen S, Zhao HM, Chen JW, Zhao YZ (2005). Enhancement of p,p '-DDT photodegradation on soil surfaces using TiO2 induced by UV-light. Chemosphere 60:266-273.
  • Sakin E and Tasdemir Y, (2016). Determination of Atmospheric PCB Level Variations in Continuously Collected Samples. Arch Environ Contam Toxicol 71:235-245.
  • Salihoglu NK, Karaca G, Salihoglu G, Tasdemir Y (2012). Removal of polycyclic aromatic hydrocarbons from municipal sludge using UV light. Desalination and Water Treatment 44:324-333.
  • Salihoğlu G, Tasdemir Y, Salihoğlu NK, Baskaya HS and Aksoy E (2013). Seasonal variations of polychlorinated biphenyl in surface soils and air-soil exchange in Bursa, Turkey. Environmental Contamination and Toxicology 65:619-634.
  • Shaban YA, El Sayed MA, El Maradny AA, Al Farawati RK, Al Zobidi MI and Khan SUM (2016). Photocatalytic removal of polychlorinated biphenyls (PCBs) using carbon-modified titanium oxide nanoparticles. Applied Surface Science 365:108-113.
  • Weber R and Sakurai T (2001). Low temperature decomposition of PCB by TiO2-based V2O5/WO3 catalyst: evaluation of the relevance of PCDF formation and insights into the first step of oxidative destruction of chlorinated aromatics. Appl Catal B-Environ 34:113-127.
  • Zhang LH, Li PJ, Gong ZQ and Li XM (2008). Photocatalytic degradation of polycyclic aromatic hydrocarbons on soil surfaces using TiO2 under UV light. J Hazard Mater 158:478-484.
  • Zhang PC, Scrudato RJ, Pagano JJ, Roberts RN (1993). Photodecomposition of Pcbs in Aqueous Systems Using TiO2 as Catalyst. Chemosphere 26:1213-1223.
  • Zhao X, Quan M, Zhao HM, Chen S, Zhao YZ and Chen JW (2004). Different effects of humic substances on photodegradation of p,p'-DDT on soil surfaces in the presence of TiO2 under UV and visible light. J Photoch Photobio A 167:177-183.

Yıl 2019, Cilt: 13 Sayı: 37, 1 - 8, 26.05.2019

Busra Tandogan Gizem Eker Sanlı

Öz

Kaynakça

  • Ahmad M, Simon MA, Sherrin A, Tuccillo ME, Ullman JL, Teel AL and Watts RJ (2011). Treatment of polychlorinated biphenyls in two surface soils using catalyzed H2O2 propagations. Chemosphere 84:855-862.
  • Brawn J F BDL, Brennan M J, Carnahan J C, Feng H, Wanger R E (1987). Polychlorinated Biphenyl Dechlorination in Aquatic Sediment. Science 236:709-712.
  • Bunce NJ, Kumar Y, Ravanal L, Safe S (1978). Cosmochemistry of chlorinated biphenyl's in ISO-octane solution. Journal of the Chemical Society-Perkins Transactions 2:880-884.
  • Cebe M (1995). Physicochemistry Volume II: Fundamental Concepts in Reaction Kinetics. Uludag University Press, Turkey.
  • Cetin B (2016). Investigation of Paths, PCBs and PCNs in soils around a Heavily Industrialized Area in Kocaeli, Turkey: Concentrations, distributions, sources and toxicological effects. Science of the Total Environment 560:160-169.
  • Dhol A (2005). An Investigation of a Photochemical Approach for the Remediation of PCB-Contaminated Soils. Master Thesis. University of Calgary, Canada.
  • Dong D, Li P, Xiaojun I, Xu C (2010). Photocatalytic degradation of phenanthrene and pyrene on soil surfaces in the presence of nanometer rutile TiO2 under UV-irradiation. Chemical Engineering Journal 158:378-383.
  • Dönmez B (2012). Research of Polychlorinated Biphenyl (PCB) Pollution in Soil Samples and Evaluation of Applicability of Limit Values. Master Thesis. Istanbul Technical University, Turkey.
  • Fasnacht MP and Blough NV (2003). Mechanisms of the aqueous photodegradation of polycyclic aromatic hydrocarbons. Environ Sci Technol 37:5767-5772.
  • Garcia R, Diaz-Somoano M, Calvo M, Lopez-Anton MA, Suarez S, Ruiz IS, Martinez-Tarazona MR (2012). Impact of a semi-industrial coke processing plant in the surrounding surface soil. Part II: PAH content Fuel Process Technol 104:245-252.
  • Guieysse B, Viklund G, Toes AC, Mattiasson B (2004). Combined UV-biological degradation of PAHs. Chemosphere 55:1493-1499.
  • Hoffmann MR, Martin ST, Choi WY, Bahnemann DW (1995). Environmental Applications of Semiconductor Photocatalysis. Chem Rev 95:69-96.
  • Ireland JC, Davila B, Moreno H, Fink SK, Tassos S (1995). Heterogeneous Photocatalytic Decomposition of Polyaromatic Hydrocarbons over Titanium-Dioxide. Chemosphere 30:965-984.
  • Jelic A, Di Fabio S, Vecchiato G, Cecchi F, Fatone F (2015). Nano-occurrence and removal of PCBs within the Europe's largest petrochemical MBR system. Water Research 83:329-336.
  • Karaca G (2013). Determination of Polycyclic Aromatic Hydrocarbon (PAHs) Levels in Treatment Sludge, Nilüfer Creek Sediment and Investigation of Removal Methods. Uludag University, Turkey.
  • Karaca G, Cindoruk SS, Tasdemir Y (2014). Migration of polycyclic aromatic hydrocarbons (PAHs) in urban treatment sludge to the air during PAH removal applications. J Air Waste Manage 64:568-577.
  • Karaca G and Tasdemir Y (2011). Effect of Diethylamine on Pah Removal from Municipal Sludge under UV Light. Fresenius Environmental Bulletin 20:1777-1784.
  • Karaca G and Tasdemir Y (2015). Application of Advanced Oxidation Processes for Polycyclic Aromatic Hydrocarbons Removal from Municipal Treatment Sludge. Clean-Soil Air Water 43:191-196.
  • Karaca G and Taşdemir Y (2015). Removal of Polycyclic Aromatic Hydrocarbons (PAHs) From Organizated Industry Dıstrıct Treatment Sludges With Photochemical Degradation: Ambient Air Applications. Journal of the Faculty of Engineering and Architecture of Gazi University 30:557-565.
  • Krauss M and Wilcke W (2002). Photochemical oxidation of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in soils - a tool to assess their degradability. J Plant Nutr Soil Sc 165:173-178.
  • Lin X, Jin Y, Wu H, Chen T, Li X, Lu S, Jiang X and Yan J (2013). Removal of PCDD/Fs and PCBs from flue gas using a pilot gas cleaning system. Journal of Environmental Sciences 25:1833-1840.
  • Lin YJ, Gupta G, Baker J (1995). Photodegradation of Polychlorinated Biphenyl Congeners Using Simulated Sunlight and Diethylamine. Chemosphere 31:3323-3344.
  • Lin YJ, Teng LS, Lee A, Chen YL (2004). Effect of photosensitizer diethylamine on the photodegradation of polychlorinated biphenyls. Chemosphere 55:879-884.
  • Meijer SN, Ockenden WA, Sweetman A, Breivik K, Grimalt JO, Jones KC (2003). Global distribution and budget of PCBs and CB in background surface soils: Implications for sources and environmental processes. Environ Sci Technol 37:667-672.
  • Melnyk A, Dettlaff A, Kuklinska K, Namiesnik J, Wolska L (2015). Concentration and sources of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in surface soil near a municipal solid waste (MSW) landfill. Science of the Total Environment 530:18-27.
  • Miller JS and Olejnik D (2001). Photolysis of polycyclic aromatic hydrocarbons in water. Water Res 35:233-243.
  • Ogulmus R (2012). Territories Polychlorinated Biphenyls (PCBs) Regional and Seasonal Conditions. Master Thesis. Uludag University, Turkey.
  • Ortiz R, Vega S, Gutierrez R, Gibson R, Schettino B and Ramirez ML (2012). Presence of Polycyclic Aromatic Hydrocarbons (PAHs) in Top Soils from Rural Terrains in Mexico City. Bulletin of Environmental Contamination and Toxicology 88:428-432.
  • Pleskov YV, Fujishima A, Hashimoto K and Watanabe T (1999). TiO2 photocatalysis: Fundamentals and applications, Tokyo: Bks, Inc., Russ. J Electrochem 35:1137-1138.
  • Quan X, Zhao X, Chen S, Zhao HM, Chen JW, Zhao YZ (2005). Enhancement of p,p '-DDT photodegradation on soil surfaces using TiO2 induced by UV-light. Chemosphere 60:266-273.
  • Sakin E and Tasdemir Y, (2016). Determination of Atmospheric PCB Level Variations in Continuously Collected Samples. Arch Environ Contam Toxicol 71:235-245.
  • Salihoglu NK, Karaca G, Salihoglu G, Tasdemir Y (2012). Removal of polycyclic aromatic hydrocarbons from municipal sludge using UV light. Desalination and Water Treatment 44:324-333.
  • Salihoğlu G, Tasdemir Y, Salihoğlu NK, Baskaya HS and Aksoy E (2013). Seasonal variations of polychlorinated biphenyl in surface soils and air-soil exchange in Bursa, Turkey. Environmental Contamination and Toxicology 65:619-634.
  • Shaban YA, El Sayed MA, El Maradny AA, Al Farawati RK, Al Zobidi MI and Khan SUM (2016). Photocatalytic removal of polychlorinated biphenyls (PCBs) using carbon-modified titanium oxide nanoparticles. Applied Surface Science 365:108-113.
  • Weber R and Sakurai T (2001). Low temperature decomposition of PCB by TiO2-based V2O5/WO3 catalyst: evaluation of the relevance of PCDF formation and insights into the first step of oxidative destruction of chlorinated aromatics. Appl Catal B-Environ 34:113-127.
  • Zhang LH, Li PJ, Gong ZQ and Li XM (2008). Photocatalytic degradation of polycyclic aromatic hydrocarbons on soil surfaces using TiO2 under UV light. J Hazard Mater 158:478-484.
  • Zhang PC, Scrudato RJ, Pagano JJ, Roberts RN (1993). Photodecomposition of Pcbs in Aqueous Systems Using TiO2 as Catalyst. Chemosphere 26:1213-1223.
  • Zhao X, Quan M, Zhao HM, Chen S, Zhao YZ and Chen JW (2004). Different effects of humic substances on photodegradation of p,p'-DDT on soil surfaces in the presence of TiO2 under UV and visible light. J Photoch Photobio A 167:177-183.
Toplam 38 adet kaynakça vardır.

Ayrıntılar

Birincil Dil İngilizce
Konular Tarımsal Biyoteknoloji (Diğer)
Bölüm Makaleler
Yazarlar

Busra Tandogan

Gizem Eker Sanlı

Yayımlanma Tarihi 26 Mayıs 2019
Yayımlandığı Sayı Yıl 2019 Cilt: 13 Sayı: 37

Kaynak Göster

APA Tandogan, B., & Eker Sanlı, G. (2019). Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications. Journal of Biological and Environmental Sciences, 13(37), 1-8.
AMA Tandogan B, Eker Sanlı G. Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications. JBES. Mayıs 2019;13(37):1-8.
Chicago Tandogan, Busra, ve Gizem Eker Sanlı. “Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications”. Journal of Biological and Environmental Sciences 13, sy. 37 (Mayıs 2019): 1-8.
EndNote Tandogan B, Eker Sanlı G (01 Mayıs 2019) Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications. Journal of Biological and Environmental Sciences 13 37 1–8.
IEEE B. Tandogan ve G. Eker Sanlı, “Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications”, JBES, c. 13, sy. 37, ss. 1–8, 2019.
ISNAD Tandogan, Busra - Eker Sanlı, Gizem. “Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications”. Journal of Biological and Environmental Sciences 13/37 (Mayıs 2019), 1-8.
JAMA Tandogan B, Eker Sanlı G. Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications. JBES. 2019;13:1–8.
MLA Tandogan, Busra ve Gizem Eker Sanlı. “Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications”. Journal of Biological and Environmental Sciences, c. 13, sy. 37, 2019, ss. 1-8.
Vancouver Tandogan B, Eker Sanlı G. Removal of Polychlorinated Biphenyls (PCBS) From Soils Using Additives: Ambient Air Applications. JBES. 2019;13(37):1-8.

Journal of Biological and Environmental Sciences is the official journal of Bursa Uludag University

Bursa Uludag University, Gorukle Campus, 16059, Bursa, Türkiye.